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Sarte, P. M.; Cruz-Kan, K.; Ortiz, B. R.; Hong, K. H.; Bordelon, M. M.; Reig-i-Plessis, D.; Lee, M.; Choi, E. S.; Stone, M. B.; Calder, S.; et al (, npj Quantum Materials)Abstract The magnetic ground state of the pyrochlore Yb 2 GaSbO 7 has not been established. The persistent spin fluctuations observed by muon spin-relaxation measurements at low temperatures have not been adequately explained for this material using existing theories for quantum magnetism. Here we report on the synthesis and characterisation of Yb 2 GaSbO 7 to revisit the nature of the magnetic ground state. Through DC and AC magnetic susceptibility, heat capacity, and neutron scattering experiments, we observe evidence for a dynamical ground state that makes Yb 2 GaSbO 7 a promising candidate for disorder-induced spin-liquid or spin-singlet behaviour. This state is quite fragile, being tuned to a splayed ferromagnet in a modest magnetic field μ 0 H c ~ 1.5 T.more » « less
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Zhang, H; Liu, S; Nelson, C S; Bezmaternykh, L N; Chen, Y-S; Wang, S G; Lobo, R P; Page, K; Matsuda, M; Pajerowski, D M; et al (, Journal of Physics: Condensed Matter)
